Bentonitic earth catalyzed rearrangement of aryl 1, 1??dimethylpropargyl ethers. Synthesis of 2, 2??dimethyl??2H??1??benzopyrans
R Cruz??Almanza, F Pérez??Flores…
Index: Cruz-Almanza, Raymundo; Perez-Flores, Francisco; Brena, Leonardo; Tapia, Eva; Ojeda, Reyna; Fuentes, Aidee Journal of Heterocyclic Chemistry, 1995 , vol. 32, # 1 p. 219 - 222
Full Text: HTML
Citation Number: 8
Abstract
Abstract Mexican Bentonitic earth (Tonsil) catalyzed the Claisen rearrangement of aryl 1, 1- dimethylpropargyl ethers under mild conditions to provide 2, 2-dimethyl-2H-1-benzopyrans. The synthesis of encecalin 2f and desmethoxyencecalin 2i, two biologically active products among other natural products (2b, 2e) was performed by this procedure.
Related Articles:
[North, Jeffrey T.; Kronenthal, David R.; Pullockaran, Annie J.; Real, Sharon D.; Chen, Helen Y. Journal of Organic Chemistry, 1995 , vol. 60, # 11 p. 3397 - 3400]
[Kawase, Yoshiyuki; Yamaguchi, Seiji; Horita, Hisanori; Takeno, Junko; Kameyama, Hideaki Bulletin of the Chemical Society of Japan, 1982 , vol. 55, # 4 p. 1153 - 1155]
[Hepworth, John D.; Jones, Terry K.; Livingstone, Robert Tetrahedron, 1981 , vol. 37, # 15 p. 2613 - 2616]