Fabrication and Deterministic Transfer of High-Quality Quantum Emitters in Hexagonal Boron Nitride

Tobias Vogl, Geoff Campbell, Ben C. Buchler, Yuerui Lu, Ping Koy Lam

Index: 10.1021/acsphotonics.8b00127

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Abstract

Color centers in solid state crystals have become a frequently used system for single-photon generation, advancing the development of integrated photonic devices for quantum optics and quantum communication applications. In particular, defects hosted by two-dimensional (2D) hexagonal boron nitride (hBN) are a promising candidate for next-generation single-photon sources, due to its chemical and thermal robustness and high brightness at room temperature. The 2D crystal lattice of hBN allows for a high extraction efficiency and easy integration into photonic circuits. Here we develop plasma etching techniques with subsequent high-temperature annealing to reliably create defects. We show how different fabrication parameters influence the defect formation probability and the emitter brightness. A full optical characterization reveals the higher quality of the created quantum emitters, represented by a narrow spectrum, short excited state lifetime, and high single-photon purity. We also investigated the photostability on short and very long time scales. We utilize a wet chemically assisted transfer process to reliably transfer the single-photon sources onto arbitrary substrates, demonstrating the feasibility for the integration into scalable photonic quantum information processing networks.