Continuous-Flow Preparation and Use of β-Chloro Enals Using the Vilsmeier Reagent

L Pellegatti, SL Buchwald

Index: Pellegatti, Laurent; Buchwald, Stephen L. Organic Process Research and Development, 2012 , vol. 16, # 8 p. 1442 - 1448

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Citation Number: 11

Abstract

The Vilsmeier reagent is used in the preparation of a wide variety of heterocycles, such as pyrazoles, via formation of β-chloroacrolein intermediates. However, use of this extremely reactive reagent on large scale requires special precautions to avoid potentially dangerous exotherms. This article describes the safe preparation at room temperature of the Vilsmeier reagent under flow conditions for the formation of β-chloroacroleins and 3- ...

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