Formal total synthesis of shikonin via Dötz benzannulation
SR Pulley, B Czakó
Index: Pulley, Shon R.; Czako, Barbara Tetrahedron Letters, 2004 , vol. 45, # 28 p. 5511 - 5514
Full Text: HTML
Citation Number: 24
Abstract
The Dötz benzannulation reaction provides mild conditions for the construction of highly functionalized aromatic compounds. We have utilized this method for the formal total synthesis of shikonin. The key step in our approach is the application of the Dötz benzannulation reaction between Fischer a chromium carbene complex and an optically active alkyne for the construction of the aromatic skeleton. This is followed by protecting ...
Related Articles:
[Bochicchio, Antonella; Chiummiento, Lucia; Funicello, Maria; Lopardo, Maria Teresa; Lupattelli, Paolo Tetrahedron Letters, 2010 , vol. 51, # 21 p. 2824 - 2827]
[Garst, Michael E.; Frazier, Janice D. Journal of Organic Chemistry, 1987 , vol. 52, # 3 p. 446 - 448]