Rhodium Enalcarbenoids: Direct Synthesis of Indoles by Rhodium (II)??Catalyzed [4+ 2] Benzannulation of Pyrroles

…, H Chennamsetti, BS Lad, S Katukojvala

Index: Dawande, Sudam Ganpat; Kanchupalli, Vinaykumar; Kalepu, Jagadeesh; Chennamsetti, Haribabu; Lad, Bapurao Sudam; Katukojvala, Sreenivas Angewandte Chemie - International Edition, 2014 , vol. 53, # 16 p. 4076 - 4080 Angew. Chem., 2014 , vol. 126, # 16 p. 4160 - 4164,5

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Citation Number: 24

Abstract

Abstract Disclosed herein is the design of an unprecedented electrophilic rhodium enalcarbenoid which results from rhodium (II)-catalyzed decomposition of a new class of enaldiazo compounds. The synthetic utility of these enalcarbenoids has been successfully demonstrated in the first transition-metal-catalyzed [4+ 2] benzannulation of pyrroles, thus leading to substituted indoles. The new benzannulation has been applied to the efficient ...

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